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Aluminum- and iron-based coagulation for in-situ removal of dissolved organic carbon, disinfection byproducts, mercury and other constituents from agricultural drain water

Journal of Geochemical Exploration (Elsevier) | May 9th, 2019

Summary

Agricultural production on wetland soils can be significant sources of dissolved organic carbon (DOC), disinfection byproduct precursors, mercury and nutrients to downst

Agricultural production on wetland soils can be significant sources of dissolved organic carbon (DOC), disinfection byproduct precursors, mercury and nutrients to downstream water bodies and accelerate land subsidence. Presented as a potential solution for in-situ water quality improvement and land subsidence mitigation, chemically enhanced treatment wetlands (CETWs) were used to leverage both coagulation and wetland processes. In this study, we evaluated the performance of coagulants ferric sulfate (Fe dosing) and polyaluminum chloride (Al dosing) to remove pollutants from agricultural drain water using the coagulation system designed for CETWs. Both coagulation treatments removed over 70% DOC from source waters, resulting in removal efficiencies (mg-DOC removed per mg-metal dosed) of 1 under Al dosing and 0.5 under Fe dosing. Coagulation by both treatments preferentially removed UV254 active compounds compared to the bulk DOC concentration, suggesting coagulation targeted aromatics more effectively. Phosphates and haloacetic acids were also removed more readily, whereas trihalomethanes, dissolved organic nitrogen and filtered mercury species were removed at similar or lower rates than DOC. Dissolved inorganic nitrogen was not amenable to coagulation and removal was not observed. Freundlich, Langmuir and Monod models explained 33% of the variance in DOC removal for Al dosing and 78–89% of the variance for Fe dosing. All three models indicated Al dosing had higher removal efficiency and affinity for DOC than Fe dosing under study conditions, but when used to predict maximum removal efficiency there was no cohesiveness between the three models due to different model assumptions. Consideration of fluorescence dissolved organic matter and UV254 as surrogates for DOC concentration showed both were equally suitable before coagulant application, but as surrogates after coagulant application, neither could be deemed more fit as a surrogate since both were shown suitable for different treatment scenarios.

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Anthropogenic and geologic causes of anomalously high uranium concentrations in groundwater used for drinking water supply in the southeastern San Joaquin Valley, CA

Journal of Hydrology (Elsevier) | October 1st, 2019

Summary

Concentrations of uranium (U) >30 µg/L in groundwater are relatively uncommon in drinking water in the United States but can be of concern in those areas where comp

Concentrations of uranium (U) >30 µg/L in groundwater are relatively uncommon in drinking water in the United States but can be of concern in those areas where complex interactions of aquifer materials and anthropogenic alterations of the natural flow regime mobilize U. High concentrations (>30 µg/L) of U in the southeastern San Joaquin Valley, California, USA, have been detected in 24 percent of 257 domestic, irrigation, and public-supply wells sampled across an approximately 110,000 km2 area. In this study we evaluated mechanisms for mobilization of U in the San Joaquin Valley proposed in previous studies, confirming mobilization by HCO3 and refuting mobilization by NO3 and we refined our understanding of the geologic sources of U to the scale of individual alluvial fans. The location of high concentrations depends on the interactions of geological U sources from fluvial fans that originate in the Sierra Nevada to the east and seepage of irrigation water that contains high concentrations of HCO3 that leaches U from the sediments. In addition, interactions with PO4 from fertilized irrigated fields may sequester U in the aquifer. Principal component analysis of the data demonstrates that HCO3 and ions associated with high total dissolved solids in the aquifer and the percentage of agriculture near the well sampled are associated with high U concentrations. Nitrate concentrations do not appear to control release of U to the aquifer. Age dating of the groundwater and generally increasing U concentrations of the past 25  years in resampled wells where irrigation is prevalent suggests that high U concentrations are associated with younger water, indicating that irrigation of fields over the past 100  years has significantly contributed to increasing concentrations and mobilizing U. In some places, the groundwater is supersaturated with uranyl-containing minerals, as would be expected in roll front deposits. In general, the interaction of natural geological sources high in U, the anthropogenically driven addition of HCO3 and possibly phosphate fertilizer, control the location and concentration of U in each individual fluvial fan, but the addition of nitrate in fertilizer does not appear control the location of high U. These geochemical interactions are complex but can be used to determine controls on anomalously high U in alluvial aquifers.

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Anthropogenic debris in seafood: Plastic debris and fibers from textiles in fish and bivalves sold for human consumption

Nature Portfolio (Springer Nature) | September 24th, 2015

Summary

The ubiquity of anthropogenic debris in hundreds of species of wildlife and the toxicity of chemicals associated with it has begun to raise concerns regarding the presenc

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Anthropogenic Stressors and Changes in the Clear Lake Ecosystem as Recorded in Sediment Cores

Ecological Society of America (Wiley) | December 1st, 2008

Summary

Sediment cores were collected to investigate multiple stresses on Clear Lake, California, USA, through the period of European occupation to the present day. Earlier wor

Sediment cores were collected to investigate multiple stresses on Clear Lake, California, USA, through the period of European occupation to the present day. Earlier workers suggested the hypothesis that the use of mechanized earthmoving equipment, starting in the 1920s and 1930s, was responsible for erosion, mercury (Hg) contamination, and habitat loss stresses. Cores (;2.5 m in depth) were collected in 1996 and 2000 from each of the three arms of the lake. Carbon-14 dating suggests that these cores represent as much as 3000 years of the lake’s history, beginning long before European settlement. Total mercury (TotHg) and methylmercury (MeHg), dry matter, water, carbon, nitrogen, phosphorus, sulfur, and the stable isotopes 13C and 15N were measured at 5-cm intervals. Nearly all parameters show major changes at depths of 58–135 cm, beginning at ca. 1927 (dated with 210Pb). Accepting this date for concomitant major changes in seven cores yields an estimated 8.6 mm/yr average sedimentation rate after 1927. Pre-1927 sedimentation rates were ;1 mm/yr. Total mercury and MeHg, dry matter, phosphorus, and 15N increase significantly, whereas nitrogen, sulfur, carbon, and water content decrease significantly above the 1927 horizon. Both TotHg and MeHg show extremely large increases (roughly 10-fold) above the 1927 horizon. A peak in inorganic deposition rate and minimum values for percentage of water is present at depths corresponding to ca. 1970. Interestingly, the first 75 years of European settlement in the Clear Lake basin (including the most productive years of the Sulphur Bank Mercury Mine) appeared to have had undetectable effects on lake cores. Changes since 1927 were dramatic. The large increase in Hg beginning about 1927 corresponds to the use of heavy equipment to exploit the ore deposit at the mine using open-pit methods. Increases in sediment deposition from increased earthmoving in the basin and sulfate loading from the mine are the most likely explanations for the dramatic changes seen in the post-1927 sections of the cores.

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Anticipating Environmental and Environmental-Health Implications of Extreme Storms: ARkStorm Scenario

American Society of Civil Engineers (ASCE) | July 22nd, 2015

Summary

The ARkStorm Scenario predicts that a prolonged winter storm event across California would cause extreme precipitation, flooding, winds, physical damages, and e

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Arsenic in California Drinking Water

Environmental Integrity Project | September 15th, 2016

Summary

More than three years after the U.S. Environmental Protection Agency found California in noncompliance with the federal Safe Drinking Water Act, 95 community water system

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Arsenic, chromium, uranium, and vanadium in rock, alluvium, and groundwater, Mojave River and Morongo Areas, western Mojave Desert, southern California

U.S. Geological Survey (USGS) | October 16th, 2023

Summary

Trace elements within groundwater that originate from aquifer materials and pose potential public-health hazards if consumed are known as geogenic contaminants. The geoge

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Arsenic, Chromium, Uranium, and Vanadium in Rock, Arsenic, Chromium, Uranium, and Vanadium in Rock, Alluvium, and Groundwater, Mojave River and Morongo Alluvium, and Groundwater, Mojave River and Morongo Areas, Western Mojave Desert, Southern California

U.S. Geological Survey (USGS) | October 16th, 2023

Summary

Trace elements within groundwater that originate from aquifer materials and pose potential public-health hazards if consumed are known as geogenic contaminants. The geoge

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Bioaccumulation of Pollutants in California Waters: A Review of Historic Data and Assessment of Impacts on Fishing and Aquatic Life

San Francisco Estuary Institute (SFEI) | October 24th, 2007

Summary

This report was written for the State Water Resources Control Board’s Surface Water Ambient Monitoring Program (SWAMP) as a step toward the development of an im

This report was written for the State Water Resources Control Board’s Surface Water Ambient Monitoring Program (SWAMP) as a step toward the development of an improved bioaccumulation monitoring program for California. The report provides a review of bioaccumulation monitoring data generated under three historic State Board programs (the Toxic Substances Monitoring Program, the State Mussel Watch Program, and the Coastal Fish Contamination Program) and other major bioaccumulation studies since 1970. Future monitoring will be guided by assessment questions developed for the SWAMP. The objective of this report was to evaluate how well the historic data from the State Board programs and from other major monitoring efforts since 1970 address these questions. This exercise has provided a substantial amount of information about present and historical impacts of pollutant bioaccumulation on shing and aquatic life in California, and has also highlighted areas where improved sampling approaches can better address the assessment questions. Present concentrations of pollutants in many California water bodies are high enough to cause concern for possible effects on human health and to have a significant impact on the fishing beneficial use. Consumption advisories, 303(d) listings, and the bioaccumulation database as a whole provide three indices of the status of this impact. Consumption advisories exist for an increasing number of water bodies, but these represent only a fraction of the areas likely to need them. Lack of suitable data is a major impediment to developing advice for additional water bodies. A US E.P.A. evaluation of the 2002 303(d) List indicated that large portions of the state had not been assessed, especially rivers and coastline. Most of the lake area in the state (61%) had been assessed, and a relatively small percentage of the total area (6%) was classified as impaired. Assessment of lakes, however, has focused primarily on the largest lakes, leaving the vast majority of smaller lakes unsampled. Many of these small lakes are near population centers and are popular for shing. Bays and estuaries had been thoroughly assessed (98% of the area) and 93% of the total area was impaired. Evaluation of the most recent monitoring data (collected from 1998-2003) indicates that, for the locations sampled, 32% had low concentrations of pollutants, 42% had moderate concentrations, 18% had high concentrations, and 8% had very high concentrations (Figure 1). Concentrations in the low category are in a range where consumption is generally encouraged by the California Office of Environmental Health Hazard Assessment (OEHHA) (Klasing and Brodberg 2006). OEHHA is the agency responsible for managing health risks due to contaminated sport fish in California. Concentrations in the very high category are in a range where OEHHA discourages consumption (Klasing and Brodberg 2006). Lakes assigned to the moderate, high, or very high concentration categories were primarily affected by mercury, with PCBs also playing a lesser role.

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Bioanalytical and chemical-specific screening of contaminants of concern in three California (USA) watersheds

Heliyon (Elsevier) | May 5th, 2022

Summary

To broaden the scope of contaminants monitored in human-impacted riverine systems, water, sediment, and treated wastewater effluent were analyzed using receptor-based cel

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Aluminum- and iron-based coagulation for in-situ removal of dissolved organic carbon, disinfection byproducts, mercury and other constituents from agricultural drain water

Anthropogenic and geologic causes of anomalously high uranium concentrations in groundwater used for drinking water supply in the southeastern San Joaquin Valley, CA

Anthropogenic debris in seafood: Plastic debris and fibers from textiles in fish and bivalves sold for human consumption

Anthropogenic Stressors and Changes in the Clear Lake Ecosystem as Recorded in Sediment Cores

Anticipating Environmental and Environmental-Health Implications of Extreme Storms: ARkStorm Scenario

Arsenic in California Drinking Water

Arsenic, chromium, uranium, and vanadium in rock, alluvium, and groundwater, Mojave River and Morongo Areas, western Mojave Desert, southern California

Arsenic, Chromium, Uranium, and Vanadium in Rock, Arsenic, Chromium, Uranium, and Vanadium in Rock, Alluvium, and Groundwater, Mojave River and Morongo Alluvium, and Groundwater, Mojave River and Morongo Areas, Western Mojave Desert, Southern California

Bioaccumulation of Pollutants in California Waters: A Review of Historic Data and Assessment of Impacts on Fishing and Aquatic Life

Bioanalytical and chemical-specific screening of contaminants of concern in three California (USA) watersheds

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